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recently did a poll of top Superhero movies. Here is the list:
Dark Knight, The (Bale)
Iron Man (Downey Jr.)
Batman Begins (Bale)
Spider-Man (Maguire)
X-Men (Stewart, Jackman, etc.)
Kick-Ass (Johnson, Moretz)
X-Men: First Class (McAvoy, etc.)
Watchmen (Crudup, Akerman, etc.)
X-Men 2: X-Men United (Stewart, Jackman, etc.)
Spider-Man 2 (Maguire)
Batman (Keaton)
I, for one, fucking hated the Spider-Man movies but maybe I need to see them again. Other than that - I may not agree with the order - but it captures most of the best superhero movies.